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Jaquen is a bigger departure, a more fleshed out character which I think an actor like patinkin would favor and ultimately not such a big role that he couldn't potentially play the role.
While you are probably correct PG patinkin is certaintly good enough to affect an accent Also Jaquen is Pentoshi supposedly if I remember right so a different accent could be in order.
lordnedshead i think mandy patinkin would be great for syrio. he'd basically be revisiting his role as the spaniard in "Princess Bride". but he's got his own tv show so I don't see it happening.